Morning, so from what I can understand, the Along Velocity mode should be what you’re looking for.
If we look at the computed source code of this block, it considers the Particle’s velocity and uses it for the Y-axis used to align particles. Now the Z-axis, which is the particle’s facing vector, uses the Camera’s position.
axisY = normalize(velocity);
axisZ = position - GetViewVFXPosition();
axisX = VFXSafeNormalizedCross(axisY, axisZ, float3(1,0,0));
axisZ = cross(axisX,axisY);
The fact that you are using an Isometric camera shouldn’t be a problem here.
Now, I tried on my side, and I think that the issue that you’re having is related to “perspective impression” or the lack of it. The result would be the same with a perspective camera and a tiny FOV, as the depth impression is being squashed and everything appears like it’s on the same plane.
When looking at the Iso view, something seems wrong at first, but it’s an optical illusion due to the lack of depth information. Our eyes have trouble understanding on which depth layer are the different particles, and their velocity and Y-axis seem to be aligned on the Camera plane.
Now, If I just display my emitter source gizmo, suddenly particles alignments depth are more “readable”.

So, I maybe what you could do is to try to reinforce the depth/layer impression of your particles.
They are several ways to do this, and here is a short list that could be tested:
- Add a small clouds/source object on top of your Rain.
- Reinforce the depth by creating layers
of rain instead of spawning uniformly in a volume.
- Modulate the Size or Color and/or Alpha based on those layers.
- Lit or Fake lighting so that particles that are supposed to be in shadow are less visible, making it more obvious where they stand in your depth.
- Add Spawn splashes/drip at collision to help make some connection with the environment.
These are some ways that could help counter the effects that an ISO Cam can have on depth perception.
I’ve made a quick attempt to apply those solutions, and while it’s definitely more work, it “felt” better.

I hope that I’m not wrong and that you don’t have a more in-depth issue with your orientation. If so, please don’t hesitate to continue this conversation.
Wish you a day without rain.